Faculty of Engineering

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Author: search.filters.author.Thambiliyagodage, CHas files: Yes

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    PublicationOpen Access
    Influence of ageing of graphene oxide on the properties and morphology of cement mortar
    (Nature Research, 2025-12-02) Suganthiny,G; Thambiliyagodage, C; Perera, S. V. T. J; Rajapakse, R. K. N. D
    Past studies show that Graphene Oxide (GO) enhances the structural properties of cement composites. However, GO reduces its chemical characteristics with ageing. This study determines the effects of the age of commercial and laboratory-produced GO on cementitious composites. The study considered GO of up to 35 weeks of age, and specimens were chemically characterised using various techniques. The ageing effects were evaluated using consistency, initial setting time, compressive strength, splitting tensile strength, and water absorption. The composite’s thermal resistance was also tested. GO was found to have a shelf life of 13 weeks from production to achieve favourable results. The morphology of the cement mortar was studied to determine the reason for the change in performance with GO age. This study confirms that the carbon-to-oxygen ratio (C/O) and the disorder of graphene oxide sheets (ID/IG ratio), along with the number of GO layers, govern the performance of GO-incorporated cement composites. Both ratios increase with GO age. Aged GOs in mortar increased the mean pore radius and reduced the surface area. Mortar samples with aged GOs have ettringite peaks, while early-age GO-containing samples lack ettringite peaks. Despite reduced mechanical performance with age, all mortar samples remained thermally stable at higher temperatures.
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    PublicationOpen Access
    Development of Silica-Copper Nanocomposite for Water Purification
    (SLIIT, 2022-02-11) Angappan, S; Karunaratne, M; Thambiliyagodage, C
    Water pollution is one of the serious concerns across the world at the moment. Industrial wastewater significantly contributes to the negative impacts caused by water pollution. Textile industries discharge large amounts of effluents into water streams with little or no treatment of the discharge because wastewater treatment is an expensive process. Thus, there exists a need for a cheap and effective way to treat textile effluent that contains dyes before being discharged. A high purity silica-based Nano-adsorbent was synthesized by using rice husk as the commercially available main cheap precursor. Copper-loaded silica nanoparticles were successfully functionalized with 3-aminopropyl triethoxysilane (APTES) via the sol-gel pathway to enhance the adsorption performance of organic dyes from textile effluent. The performance of produced Nano-adsorbent was evaluated by using methylene blue as waste adsorbate. As synthesized nanomaterial was characterized by X-Ray Diffraction (XRD) and Fourier Transform Infrared (FTIR) spectroscopy, the XRD results confirmed the presence of silicon dioxide (SiO2) and paramelaconite (Cu4O3) as predicted. The FTIR confirmed the presence of Si–O stretching, N-H bending, C–H stretching, Cu–O stretching and O–H bending vibrations thereby suggesting the presence of SiO2, NH2 groups, CH2, Cu4O3 and physisorbed H2O. The optimum conditions for pH and adsorbent dosage were successfully evaluated for the adsorption process. The optimum pH at which the nanomaterial performed best was at pH 4. The optimum mass of the adsorbent that gave maximum adsorption performance was 20 mg. Kinetic studies revealed that the experimented data was in better correlation with pseudo-second-order kinetics. The outcome of this project would be of interest to textile industries looking for a cheap and effective way to treat textile wastewater